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Journal Articles

Evaluation of oxidation efficiency of hydrophobic palladium catalyst for $$^{3}$$H monitoring in radioactive gaseous waste

Furutani, Misa; Kometani, Tatsunari; Nakagawa, Masahiro; Ueno, Yumi; Sato, Junya; Iwai, Yasunori*

Hoken Butsuri (Internet), 55(2), p.97 - 101, 2020/06

https://doi.org/10.5453/jhps.55.97

Herein, an oxidation catalyst was introduced after heating it to 600$$^{circ}$$C to oxidize tritium gas (HT) existing in exhaust into tritiated water vapor (HTO). This study aims to establish a safer $$^{3}$$H monitoring system by lowering the heating temperature required for the catalyst. In these experiments, which were conducted in the Nuclear Science Research Institute, Japan Atomic Energy Agency, cupric oxide, hydrophobic palladium/silicon dioxide (Pd/SiO$$_{2}$$), and platinum/aluminum oxide (Pt/Al$$_{2}$$O$$_{3}$$) catalysts were ventilated using standard hydrogen gas. After comparing the oxidation efficiency of each catalyst at different temperatures, we found that the hydrophobic Pd/SiO$$_{2}$$ and Pt/Al$$_{2}$$O$$_{3}$$ catalysts could oxidize HT into HTO at 25$$^{circ}$$C.

Journal Articles

Evaluation of oxidation efficiency of hydrophobic palladium catalyst for $$^{14}$$C monitoring in gaseous radioactive waste

Ueno, Yumi; Nakagawa, Masahiro; Sato, Junya; Iwai, Yasunori

Hoken Butsuri, 51(1), p.7 - 11, 2016/03

https://doi.org/10.5453/jhps.51.7

In the Nuclear Science Research Institute, Japan Atomic Energy Agency (JAEA), in order to oxidize $$^{14}$$C, which exists in various chemical forms in exhaust, into $$^{14}$$CO$$_{2}$$, a copper oxide (CuO) catalyst is introduced after heating to 600$$^{circ}$$C. Our goal was to establish a safer $$^{14}$$C monitoring system by lowering the heating temperature required for the catalyst; therefore, we developed a new hydrophobic palladium/silicon dioxide (Pd/SiO$$_{2}$$) catalyst that makes the carrier's surface hydrophobic. In these experiments, catalysts CuO, platinum/aluminum oxide (Pt/Al$$_{2}$$O$$_{3}$$), palladium/zirconium dioxide (Pd/ZrO$$_{2}$$), hydrophobic Pd/SiO$$_{2}$$, and hydrophilic Pd/SiO$$_{2}$$ were ventilated with standard methane gas, and we compared the oxidation efficiency of each catalyst at different temperatures. As a result, we determined that the hydrophobic Pd/SiO$$_{2}$$ catalyst had the best oxidation efficiency. By substituting the currently used CuO catalyst with the hydrophobic Pd/SiO$$_{2}$$ catalyst, we will be able to lower the working temperature from 600$$^{circ}$$C to 300$$^{circ}$$C and improve the safety of the monitoring process.

JAEA Reports

None

; ; Kano, Yutaka; ;

PNC TN8520 94-008, 37 Pages, 1994/09

PNC-TN8520-94-008.pdf:1.91MB

None

Journal Articles

The statistics of meteorology for dose evaluation of crews of on atomic powered ship

;

Nihon Genshiryoku Gakkai-Shi, 23(12), p.939 - 944, 1981/00

https://doi.org/10.3327/jaesj.23.939
 Times Cited Count：0 Percentile：0.02(Nuclear Science & Technology)

no abstracts in English

Oral presentation

Evaluation of oxidation efficiency of hydrophobic palladium catalyst for $$^{14}$$C monitoring in gaseous radioactive waste in reprocessing plant and RI using facilities

Ueno, Yumi; Nakagawa, Masahiro; Sato, Junya; Iwai, Yasunori

no journal, , 

no abstracts in English

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